光谱学与光谱分析 |
|
|
|
|
|
The Remove Characteristics of Dissolved Organic Matter in Landfill Leachate During the Treatment Process |
HE Xiao-song1, 2, YU Jing3, XI Bei-dou2*, JIANG Yong-hai2, ZHANG Jin-bao2, LI Dan2, PAN Hong-wei2, LIU Hong-liang2 |
1. School of Environment, Beijing Normal University, Beijing 100875, China 2. Laboratory of Water Environmental System Engineering, Chinese Research Academy of Environmental Science, Beijing 100012, China 3. State Key Laboratory of Geological Hazard Prevention and Geological Environment Protection, Chengdu University of Technology, Chengdu 610059, China |
|
|
Abstract In order to investigate remove characteristics of dissolved organic matter in landfill leachate, leachates were sampled during the process (i.e., adjusting tank, anaerobic zone, oxidation ditch and MBR processing). Dissolved organic matter was extracted and its content and structure were characterized by fluorescence excitation-emission matrix spectra, UV-Vis specrtra and FTIR spectra. The results showed that an amount of 377.6 mg·L-1 dissolved organic carbon (DOC) was removed during the whole treatment process, and the total removal rate was up to 78.34%. The 25.56% of DOC in the adjusting tank was removed during the anaerobic zone, 41.58% of DOC in anaerobic effluent was removed during the oxidation ditch, while 50.19% of DOC in the oxidation ditch effluent decreased in the MBR process. The anaerobic process increased the content of unsaturated compound and polysaccharides in leachate DOM, which improved the leachate biochemical characteristics. The unsaturated compound and polysaccharides were removed effectively during being in oxidation ditch. Protein-like and humic-like fluorescence peaks were observed in the adjusting tank and anaerobic zone, while humic-like fluorescence peaks were just presented in the oxidation ditch and MBR processing. Protein-like and fulvic-like substances were biodegraded in the adjusting tank and anaerobic zone, while humic-like materials were removed in the MBR process.
|
Received: 2012-04-06
Accepted: 2012-07-11
|
|
Corresponding Authors:
XI Bei-dou
E-mail: xibeidou@163.net
|
|
[1] Zhang L, Li A M, Lu Y F, et al. Waste Management, 2009, 29(3): 1035. [2] He X S, Xi B D, Wei Z M, et al. Bioresouresour Technology, 2011, 102(3): 2322. [3] HE Xiao-song, XI Bei-dou, WEI Zi-min, et al(何小松, 席北斗, 魏自民, 等). Chinese Journal of Analytical Chemistry(分析化学), 2010, 38(10): 1417. [4] He X S, Xi B D, Wei Z M, et al. Journal of Hazardous Materials, 2011, 190(1-3): 293. [5] GUO Jin-song, CHEN Peng, FANG Fang, et al(郭劲松, 陈 鹏, 方 芳, 等). China Water & Wastewater(中国给水排水), 2008, 24(3): 88. [6] LI Hong-jiang, ZHAO You-cai, ZHU Ying, et al(李鸿江, 赵由才, 朱 英, 等). China Environmental Science(中国环境科学), 2008, 28(12): 1122. [7] ZENG Xiao-lan, HAN Le, DING Wen-chuan, et al(曾晓岚, 韩 乐, 丁文川, 等). Spectroscopy and Spectral Analysis(光谱学与光谱分析), 2011, 31(10): 2767. [8] XU Su-yun, HE Pin-jing, TANG Qiong-yao, et al(徐苏云, 何品晶, 唐琼瑶, 等). Research of Environmental Sciences(环境科学研究), 2010, 21(4): 1049. [9] YE Shao-fan, WU Zhi-chao, WANG Zhi-wei, et al(叶少帆, 吴志超, 王志伟, 等). Research of Environmental Sciences(环境科学研究), 2010, 23(8): 1049. [10] YE Xiu-ya,ZHOU Shao-qi,ZHENG Ke(叶秀雅, 周少奇, 郑 可). Chemical Industry and Engineering Progress(化工进展), 2011, 30(6): 1374. [11] SHI Yan, WANG Qi-shan, YUE Lin(石 岩, 王启山, 岳 琳). Journal of Beijing University of Chemical Technology(北京化工大学学报), 2008, 35(6): 84. [12] QIN Fang-hui, WU Yan-yu, YE Xiu-ya, et al(覃芳慧, 吴彦瑜, 叶秀雅, 等). Chinese Journal of Environmental Engineering(环境工程学报), 2010, 4(12): 2709. [13] Zsolnay A, Baigar E, Jimenez M, et al. Chemosphere, 1999, 38, 45. [14] Chen W, Westerhoff P, Leenheer J A, et al. Environmental Science & Technology 2003, 37(24): 5701. [15] Marhuenda-Egea F C, Martínez-Sabater E, Jordá J, et al. Chemosphere, 2007, 68(2): 301. [16] Shao Z H, He P J, Zhang D Q, et al.. Journal of Hazardous Materials, 2009, 164(2-3): 1191. [17] Wu J, Zhang H, Shao L M, et al. Environmental Pollution, 2012, 162(3): 63. [18] Bu L, Wang K, Zhao Q L, et al. Journal of Hazardous Materials, 2010, 179(1-3): 1096. [19] HE Lei, WANG Zhi-wei, WU Zhi-chao(何 磊, 王志伟, 吴志超). China Environmental Science(中国环境科学), 2011, 31(2): 225. [20] Patel-Sorrentino N, Mounier S, Benaim J Y, Water Research, 2002, 36(10): 2571. [21] Baker A, Curry M. Water Research, 2004, 38(10): 2605. [22] Wang L Y, Wu F C, Zhang R Y, et al. Journal of Environmental Sciences, 2009, 21(5): 581. [23] Droussi Z, D’Orazio V, Hafidi M, et al. Journal of Hazardous Materials, 2009, 163(2-3): 1289. |
[1] |
ZHENG Hong-quan, DAI Jing-min*. Research Development of the Application of Photoacoustic Spectroscopy in Measurement of Trace Gas Concentration[J]. SPECTROSCOPY AND SPECTRAL ANALYSIS, 2024, 44(01): 1-14. |
[2] |
CHENG Jia-wei1, 2,LIU Xin-xing1, 2*,ZHANG Juan1, 2. Application of Infrared Spectroscopy in Exploration of Mineral Deposits: A Review[J]. SPECTROSCOPY AND SPECTRAL ANALYSIS, 2024, 44(01): 15-21. |
[3] |
FAN Ping-ping,LI Xue-ying,QIU Hui-min,HOU Guang-li,LIU Yan*. Spectral Analysis of Organic Carbon in Sediments of the Yellow Sea and Bohai Sea by Different Spectrometers[J]. SPECTROSCOPY AND SPECTRAL ANALYSIS, 2024, 44(01): 52-55. |
[4] |
LI Jie, ZHOU Qu*, JIA Lu-fen, CUI Xiao-sen. Comparative Study on Detection Methods of Furfural in Transformer Oil Based on IR and Raman Spectroscopy[J]. SPECTROSCOPY AND SPECTRAL ANALYSIS, 2024, 44(01): 125-133. |
[5] |
BAI Xi-lin1, 2, PENG Yue1, 2, ZHANG Xue-dong1, 2, GE Jing1, 2*. Ultrafast Dynamics of CdSe/ZnS Quantum Dots and Quantum
Dot-Acceptor Molecular Complexes[J]. SPECTROSCOPY AND SPECTRAL ANALYSIS, 2024, 44(01): 56-61. |
[6] |
XU Tian1, 2, LI Jing1, 2, LIU Zhen-hua1, 2*. Remote Sensing Inversion of Soil Manganese in Nanchuan District, Chongqing[J]. SPECTROSCOPY AND SPECTRAL ANALYSIS, 2024, 44(01): 69-75. |
[7] |
WANG Fang-yuan1, 2, HAN Sen1, 2, YE Song1, 2, YIN Shan1, 2, LI Shu1, 2, WANG Xin-qiang1, 2*. A DFT Method to Study the Structure and Raman Spectra of Lignin
Monomer and Dimer[J]. SPECTROSCOPY AND SPECTRAL ANALYSIS, 2024, 44(01): 76-81. |
[8] |
YANG Cheng-en1, 2, LI Meng3, LU Qiu-yu2, WANG Jin-ling4, LI Yu-ting2*, SU Ling1*. Fast Prediction of Flavone and Polysaccharide Contents in
Aronia Melanocarpa by FTIR and ELM[J]. SPECTROSCOPY AND SPECTRAL ANALYSIS, 2024, 44(01): 62-68. |
[9] |
LIU Zhen1*, LIU Li2*, FAN Shuo2, ZHAO An-ran2, LIU Si-lu2. Training Sample Selection for Spectral Reconstruction Based on Improved K-Means Clustering[J]. SPECTROSCOPY AND SPECTRAL ANALYSIS, 2024, 44(01): 29-35. |
[10] |
YANG Chao-pu1, 2, FANG Wen-qing3*, WU Qing-feng3, LI Chun1, LI Xiao-long1. Study on Changes of Blue Light Hazard and Circadian Effect of AMOLED With Age Based on Spectral Analysis[J]. SPECTROSCOPY AND SPECTRAL ANALYSIS, 2024, 44(01): 36-43. |
[11] |
GAO Feng1, 2, XING Ya-ge3, 4, LUO Hua-ping1, 2, ZHANG Yuan-hua3, 4, GUO Ling3, 4*. Nondestructive Identification of Apricot Varieties Based on Visible/Near Infrared Spectroscopy and Chemometrics Methods[J]. SPECTROSCOPY AND SPECTRAL ANALYSIS, 2024, 44(01): 44-51. |
[12] |
ZHENG Pei-chao, YIN Yi-tong, WANG Jin-mei*, ZHOU Chun-yan, ZHANG Li, ZENG Jin-rui, LÜ Qiang. Study on the Method of Detecting Phosphate Ions in Water Based on
Ultraviolet Absorption Spectrum Combined With SPA-ELM Algorithm[J]. SPECTROSCOPY AND SPECTRAL ANALYSIS, 2024, 44(01): 82-87. |
[13] |
XU Qiu-yi1, 3, 4, ZHU Wen-yue3, 4, CHEN Jie2, 3, 4, LIU Qiang3, 4 *, ZHENG Jian-jie3, 4, YANG Tao2, 3, 4, YANG Teng-fei2, 3, 4. Calibration Method of Aerosol Absorption Coefficient Based on
Photoacoustic Spectroscopy[J]. SPECTROSCOPY AND SPECTRAL ANALYSIS, 2024, 44(01): 88-94. |
[14] |
LI Xin-ting, ZHANG Feng, FENG Jie*. Convolutional Neural Network Combined With Improved Spectral
Processing Method for Potato Disease Detection[J]. SPECTROSCOPY AND SPECTRAL ANALYSIS, 2024, 44(01): 215-224. |
[15] |
XING Hai-bo1, ZHENG Bo-wen1, LI Xin-yue1, HUANG Bo-tao2, XIANG Xiao2, HU Xiao-jun1*. Colorimetric and SERS Dual-Channel Sensing Detection of Pyrene in
Water[J]. SPECTROSCOPY AND SPECTRAL ANALYSIS, 2024, 44(01): 95-102. |
|
|
|
|