|
|
|
|
|
|
Geographical Origin Discrimination of Taiping Houkui Tea Using Convolutional Neural Network and Near-Infrared Spectroscopy |
CHEN Qi1,3, PAN Tian-hong2,4*, LI Yu-qiang4, LIN Hong4 |
1. School of Food and Biological Engineering, Hefei University of Technology, Hefei 230601, China
2. School of Electrical Engineering and Automation, Anhui University, Hefei 230601, China
3. Huangshan Customs Research Center for Tea Quality and Safety, Huangshan 245000, China
4. School of Electrical and Information Engineering, Jiangsu University, Zhenjiang 212013, China |
|
|
Abstract Taiping Houkui Tea, one of China’s precious tea series, occupies an important position in public consumption and the tea market. The price of Taiping Houkui tea varies greatly from different geographical origins, and accurate geographical origin discrimination is currently an important factor in promoting the green tea industry. Sensory evaluation methods that rely on the manual experience are highly subjective and poor instability and cannot be applied to the actual analysis process. As the main detection and analysis method at present, the chemical analysis method is time-consuming and laborious. More importantly, there is currently no uniform standard for the geographical origin discrimination of tea. Near-infrared spectroscopy (NIR), as non-destructive testing and analysis method, has the characteristics of fast, non-destructive, and non-polluting. However, the types and contents of main components of Taiping Houkui tea from different origins are similar, which results in the same spectral peak distributions of various samples, and conventional analysis methods are limited for selecting feature variables. As one of the typical deep learning network models, convolutional neural network (CNN) has strong feature extraction and model expression capabilities. Based on the analysis of the spectral characteristics of Taiping Houkui tea from different geographical origins, the 1-dimension CNN (1-D CNN) is used to extract the NIR features, and a discriminant method combing NIR with 1-D CNN is explored to identify the geographical origin of Taiping Houkui tea in this work. In this paper, 120 samples were collected from 6 different geographical origins. The NIR were sampled from 10 000~4 000 cm-1 and preprocessed by standard normal variate (SNV). The sample is randomly divided into a training set (84, 70%) and test set (36, 30%), and the effects of CNN structure, convolution kernel size, activation function and other parameters on the analysis results were discussed separately. As a result, a 1-D CNN model with 9-layer was constructed for the geographical origin discrimination of Taiping Houkui tea. The principal component analysis (PCA) was compared, and the Monte-Carlo method was used to evaluate the stability and robustness of the proposed method. Compared with the prediction accuracy and standard deviation of the models based on original spectral data (40.57%, 7.06) and the PCA method (31.93%, 6.96), the prediction accuracy and stability of the 1-D CNN-based geographical origin discrimination model are higher, and the average prediction accuracy and standard deviation of the testing set are 97.73% and 3.47, respectively. The comparison results demonstrate the proposed 1-D CNN model can effectively extract NIR features and has the ability to identify the geographical origins of Taiping Houkui tea, which provides an effective method for the identification and traceability analysis of the geographical origin and production of valuable tea products such as Taiping Houkui tea.
|
Received: 2020-08-04
Accepted: 2020-12-10
|
|
Corresponding Authors:
PAN Tian-hong
E-mail: thpan@live.com
|
|
[1] ZHAN Hui-bin(占辉斌). Journal of Northeast Agritultural University(东北农业大学学报), 2018, 16(1): 34.
[2] LEI Pan-deng, HUANG Jian-qin, WU Qiong, et al(雷攀登, 黄建琴, 吴 琼, 等). China Tea Processing(中国茶叶加工), 2016, 1(1): 33.
[3] PAN Tian-hong, LI Yu-qiang, CHEN Qi, et al(潘天红, 李鱼强, 陈 琦, 等). Transactions of the Chinese Society of Agricultural Engineering(农业工程学报), 2020, 36(13): 264.
[4] Li Chunlin, Guo Haowei, Zong Bangzheng, et al. Spectrochim. Acta Part A: Mol. Biomol. Spectrosc., 2019, 206: 254.
[5] Li Xiaoli, Jin Juanjuan, Sun Cahnjun, et al. Food Chem., 2019, 270: 236.
[6] Chen Xiaoyi, Chai Qinqin, Lin Ni, et al. Anal. Methods, 2019, 40(11): 5118.
[7] Satoru Hiwa, Kenya Hanawa, Ryota Tamura, et al. Comput. Intell. Neurosci., 2016, 2016(3): 1841945.
[8] Thanawin Trakoolwilaiwan, Bahareh Behboodi, Jaeseok Lee, et al. Neurophotonics, 2017, 5(1): 011008.
[9] MENG Shi-yu, HUANG Ying-lai, ZHAO Peng, et al(孟诗语, 黄英来, 赵 鹏, 等). Spectroscopy and Spectral Analysis(光谱学与光谱分析), 2020, 40(1): 284.
[10] Zou Xiaobo, Zhao Jiewen, Povey M J W, et al. Anal. Chim. Acta, 2010, 667(1): 14.
[11] Li Yuqiang, Pan Tianhong, Li Haoran, et al. J. Food Process Eng., 2020, 43(8): 13445.
[12] Ren Shaoqing, He Kaiming, Girshick Ross, et al. IEEE Trans. Pattern Anal. Mach. Intell., 2017, 39(6): 1137.
[13] Chen Quansheng, Zhao Jiewen, Sumpun Chaitep, et al. Food Chem., 2009, 113(4): 1272. |
[1] |
SHI Wen-qiang1, XU Xiu-ying1*, ZHANG Wei1, ZHANG Ping2, SUN Hai-tian1, 3, HU Jun1. Prediction Model of Soil Moisture Content in Northern Cold Region Based on Near-Infrared Spectroscopy[J]. SPECTROSCOPY AND SPECTRAL ANALYSIS, 2022, 42(06): 1704-1710. |
[2] |
WANG Xue-pei1, 2, ZHANG Lu-wei1, 2, BAI Xue-bing3, MO Xian-bin1, ZHANG Xiao-shuan1, 2*. Infrared Spectral Characterization of Ultraviolet Ozone Treatment on Substrate Surface for Flexible Electronics[J]. SPECTROSCOPY AND SPECTRAL ANALYSIS, 2022, 42(06): 1867-1873. |
[3] |
WANG Yue1, 3, 4, CHEN Nan1, 2, 3, 4, WANG Bo-yu1, 5, LIU Tao1, 3, 4*, XIA Yang1, 2, 3, 4*. Fourier Transform Near-Infrared Spectral System Based on Laser-Driven Plasma Light Source[J]. SPECTROSCOPY AND SPECTRAL ANALYSIS, 2022, 42(06): 1666-1673. |
[4] |
FENG Rui-jie1, CHEN Zheng-guang1, 2*, YI Shu-juan3. Identification of Corn Varieties Based on Bayesian Optimization SVM[J]. SPECTROSCOPY AND SPECTRAL ANALYSIS, 2022, 42(06): 1698-1703. |
[5] |
YU Zhi-rong, HONG Ming-jian*. Near-Infrared Spectral Quantitative Analysis Network Based on Grouped Fully Connection[J]. SPECTROSCOPY AND SPECTRAL ANALYSIS, 2022, 42(06): 1735-1740. |
[6] |
MENG Fan-jia1, LUO Shi1, WU Yue-feng1, SUN Hong1, LIU Fei2, LI Min-zan1*, HUANG Wei3, LI Mu3. Characteristic Extraction Method and Discriminant Model of Ear Rot of Maize Seed Base on NIR Spectra[J]. SPECTROSCOPY AND SPECTRAL ANALYSIS, 2022, 42(06): 1716-1720. |
[7] |
JI Jiang-tao1, 2, LI Peng-ge1, JIN Xin1, 2*, MA Hao1, 2, LI Ming-yong1. Study on Quantitative Detection of Tomato Seedling Robustness
in Spring Seedling Transplanting Period Based on VIS-NIR
Spectroscopy[J]. SPECTROSCOPY AND SPECTRAL ANALYSIS, 2022, 42(06): 1741-1748. |
[8] |
PENG Yan-fang1, WANG Jun1, WU Zhi-sheng2*, LIU Xiao-na3, QIAO Yan-jiang2*. NIR Band Assignment of Tanshinone ⅡA and Cryptotanshinone by
2D-COS Technology and Model Application Tanshinone Extract[J]. SPECTROSCOPY AND SPECTRAL ANALYSIS, 2022, 42(06): 1781-1785. |
[9] |
LI Qing1, 2, XU Li1, 2, PENG Shan-gui1, 2, LUO Xiao1, 2, ZHANG Rong-qin1, 2, YAN Zhu-yun3, WEN Yong-sheng1, 2*. Research on Identification of Danshen Origin Based on Micro-Focused
Raman Spectroscopy Technology[J]. SPECTROSCOPY AND SPECTRAL ANALYSIS, 2022, 42(06): 1774-1780. |
[10] |
PENG Ren-miao1, 2, XU Peng-peng2, ZHAO Yi-mo2, BAO Li-jun1, LI Cheng2*. Identification of Two-Dimensional Material Nanosheets Based on Deep Neural Network and Hyperspectral Microscopy Images[J]. SPECTROSCOPY AND SPECTRAL ANALYSIS, 2022, 42(06): 1965-1973. |
[11] |
JIANG Rong-chang1, 2, GU Ming-sheng2, ZHAO Qing-he1, LI Xin-ran1, SHEN Jing-xin1, 3, SU Zhong-bin1*. Identification of Pesticide Residue Types in Chinese Cabbage Based on Hyperspectral and Convolutional Neural Network[J]. SPECTROSCOPY AND SPECTRAL ANALYSIS, 2022, 42(05): 1385-1392. |
[12] |
JI Rong-hua1, 2, ZHAO Ying-ying2, LI Min-zan2, ZHENG Li-hua2*. Research on Prediction Model of Soil Nitrogen Content Based on
Encoder-CNN[J]. SPECTROSCOPY AND SPECTRAL ANALYSIS, 2022, 42(05): 1372-1377. |
[13] |
WANG Li-qi1, YAO Jing1, WANG Rui-ying1, CHEN Ying-shu1, LUO Shu-nian2, WANG Wei-ning2, ZHANG Yan-rong1*. Research on Detection of Soybean Meal Quality by NIR Based on
PLS-GRNN[J]. SPECTROSCOPY AND SPECTRAL ANALYSIS, 2022, 42(05): 1433-1438. |
[14] |
ZHAO Yong1, HE Men-yuan1, WANG Bo-lin2, ZHAO Rong2, MENG Zong1*. Classification of Mycoplasma Pneumoniae Strains Based on
One-Dimensional Convolutional Neural Network and
Raman Spectroscopy[J]. SPECTROSCOPY AND SPECTRAL ANALYSIS, 2022, 42(05): 1439-1444. |
[15] |
DAI Lu-lu1, YANG Ming-xing1, 2*, WEN Hui-lin1. Study on Chemical Compositions and Origin Discriminations of Hetian Yu From Maxianshan, Gansu Province[J]. SPECTROSCOPY AND SPECTRAL ANALYSIS, 2022, 42(05): 1451-1458. |
|
|
|
|