|
|
|
|
|
|
| High-Pressure Raman Study of Pyromellitic Dianhydride |
| CONG Guang-yu1, LI Dong-fei2*, LIU Jia-rui3 |
1. Department of Basic Education of Changchun Guanghua University, Changchun 130033，China
2. College of Physics, Changchun Normal University, Changchun 130032，China
3. College of Physics, Jilin Normal University, Siping 136000，China
|
|
|
|
|
Abstract Raman spectra of pyromellitic dianhydride crystal have been measured from ambient to 24 GPa, and the Raman vibrational modes of pyromellitic dianhydride have been assigned. Based on the pressure dependence of Raman mode frequencies, it can be observed that a phase transition of pyromellitic dianhydride occurred from Phase Ⅰ to Phase Ⅱ at 2 GPa. In comparing the slopes of the pressure dependence of the Raman vibrational modes between Phase Ⅰ and Phase Ⅱ, it can be found that most of the slopes of Phase Ⅰ were smaller than Phase Ⅱ. The results indicate that the sensitivity of functional groups of pyromellitic dianhydride to pressure decreases with increasing pressure, and the molecular crystal of pyromellitic dianhydride has a more compact stacking structure in phaseⅡ. Besides, we also calculated the Raman intensities ratio of the overtone of C—O stretching vibration mode (located at 1 837 cm-1) and the fundamental of C═O stretching vibration mode (located at 1 865 cm-1) and the discontinuities of the Raman intensities ratio versus pressure was observed. This behavior confirms that the pyromellitic dianhydride crystal has undergone a phase transition at 2 GPa, as mentioned above.
|
|
Received: 2023-07-06
Accepted: 2023-12-14
|
|
|
|
Corresponding Authors:
LI Dong-fei
|
|
[1] Guo R, Wang Y, Heng S, et al. Journal of Power Sources, 2019, 436: 226848.
[2] Hsiao S H, Chen Y J. European Polymer Journal, 2002, 38(4): 815.
[3] Hasegawa M, Hirano D, Fujii M, et al. Journal of Polymer Science Part A: Polymer Chemistry, 2013, 51(3): 575.
[4] O'brien K C, Koros W J, Husk G R. Journal of Membrane Science, 1988, 35(2): 217.
[5] Hsiao S H，Liao W K, et al. Liou Guey-Sheng, Polym. Chem.，2018, 9: 236.
[6] Meng P，Heng H，Sun Y, et al. Appl. Catal., B，2018, 226: 487.
[7] Akbarzadeh H, Clark S J, Ackland G J. Journal of Physics: Condensed Matter, 1993, 5(43): 8065.
[8] Pruzan P. International Journal of Materials and Product Technology, 2006, 26(3-4): 200.
[9] McMillan P F. Chemical Communications, 2003，(8): 919.
[10] Demazeau G. Journal of Physics: Condensed Matter, 2002, 14(44): 11031.
[11] Xu J A, Mao H K, Bell P M. Science, 1986, 232(4756): 1404.
[12] Mujica A, Rubio A, Muñoz A, et al. Reviews of Modern Physics, 2003, 75(3): 863.
[13] Mao H K, Xu J A, Bell P M. Journal of Geophysical Research: Solid Earth, 1986, 91(B5): 4673.
[14] Forman R A, Piermarini G J, Barnett J D, et al. Science, 1972, 176(4032): 284.
[15] Hase Y, Kawai K, Sala O. Journal of Molecular Structure, 1975, 26(2): 297.
[16] Torabi A, Song Y, Staroverov V N. The Journal of Physical Chemistry C, 2013, 117(5): 2210.
[17] Furic K, Volovšek V. Journal of Molecular Structure, 2010, 976(1-3): 174.
[18] Jayaraman A, Kourouklis G A, Van Uitert L G. Pramana, 1988, 30(3): 225.
[19] Hemley R J, Mao H K. Physical Review Letters, 1988, 61(7): 857.
[20] Perlin P, Jauberthie-Carillon C, Itie J P, et al. Physical Review B, 1992, 45(1): 83.
|
| [1] |
ZHANG Wei1, 2, FENG Wei-wei2, 3*, CAI Zong-qi2, WANG Huan-qing2, YAN Qi1, WANG Qing2, 3. Study on Recognition of Marine Microplastics Using Raman Spectra
Combined With MTF and CNN[J]. SPECTROSCOPY AND SPECTRAL ANALYSIS, 2024, 44(09): 2420-2427. |
| [2] |
ZHAO Jing-rui1, WANG Ya-min1, YUAN Yu-xun1, YU Jing1, ZHAO Ming-hui1, DONG Juan1, 3, SUN Jing-tao1, 2, 3, 4*. Study on SERS Detection of Ethyl Carbamate in Grape Spirit[J]. SPECTROSCOPY AND SPECTRAL ANALYSIS, 2024, 44(09): 2467-2475. |
| [3] |
CHEN Pei-li1, SONG Da1, 2, ZHOU Zhao-qiu1, CHEN Kai-yue1, SU Qiu-cheng1, LI Cui-qin3*. The Suppression Method of Raman Laser Thermal Effect for Sensitive
Samples[J]. SPECTROSCOPY AND SPECTRAL ANALYSIS, 2024, 44(09): 2476-2481. |
| [4] |
WEI Yu-lan, ZHANG Chen-jie, YUAN Ya-xian*, YAO Jian-lin*. In-Situ SERS Monitoring of SPR-Catalyzed Coupling Reaction of
p-Nitroiodobenzene on Noble Metal Nanoparticles[J]. SPECTROSCOPY AND SPECTRAL ANALYSIS, 2024, 44(09): 2482-2487. |
| [5] |
WAN Jing-wei1, CHEN Lei2, CHAI Wei3, KONG Wei-gang4, CUI Sheng-feng1. Identification of the Crossing Sequence of Seal Stamps and Ink of
Handwriting/Printed Documents Based on Raman Spectroscopy[J]. SPECTROSCOPY AND SPECTRAL ANALYSIS, 2024, 44(09): 2501-2505. |
| [6] |
PENG Jiao-yu1, 2, YANG Ke-li1, 2, DONG Ya-ping1, 2, FENG Hai-tao1, 2, ZHANG Bo1, 3, LI Wu1, 3. Research on the Chemical Species of Borates in Salt Lake Brine and Its Quantitative Analysis by Raman Spectroscopy[J]. SPECTROSCOPY AND SPECTRAL ANALYSIS, 2024, 44(09): 2514-2522. |
| [7] |
YE Xu1, 2, YANG Jiong2, 3*, QIU Zhi-li1, 2, YUE Zi-long1. An Exploration of Geographic Determination of Serpentine Jade by
Raman Spectroscopy Combined With Principal Component
Analysis and Linear Discriminant Analysis[J]. SPECTROSCOPY AND SPECTRAL ANALYSIS, 2024, 44(09): 2551-2558. |
| [8] |
LIU Hui-qiao1, 2, FU Jin-jin1, WANG Si-tian1, ZHANG Jia-kun1, HE Ya-nan1, CAO Kang-zhe1. Research Progress of Surface-Enhance Raman Scatting Spectrum for
miRNAs Detection[J]. SPECTROSCOPY AND SPECTRAL ANALYSIS, 2024, 44(08): 2111-2119. |
| [9] |
HUANG Ji-chong1, SONG Shao-zhong2*, LIU Chun-yu1, XU Li-Jun1, CHEN An-liang1, LU Ming1, GUO Wen-jing1, MIAO Zhuang1, LI Chang-ming1, TAN Yong1, LIU Zhe3. Research on Identification of Corn Storage Years Based on Raman
Spectroscopy[J]. SPECTROSCOPY AND SPECTRAL ANALYSIS, 2024, 44(08): 2166-2173. |
| [10] |
ZHANG Yin1, FENG Cheng-cheng2, 3, XIA Qi2, 3, HU Ting1, YUAN Li-bo1*. Deep Leaning Classification of Novel Coronavirus Raman Spectra
Enhanced by CGAN[J]. SPECTROSCOPY AND SPECTRAL ANALYSIS, 2024, 44(08): 2273-2278. |
| [11] |
MA Huan-zhen1, 4, YAN Xin-ru1, 4, XIN Ying-jian3, 4, FANG Pei-pei1, 3, 4, WANG Hong-peng3, WANG Yi-an1, 4, DUAN Ming-kang3, 4, JIA Jian-jun3, HE Ji-ye2*, WAN Xiong1, 3*. Blood Identification Based on AFSA-SVM Dynamic Spectra[J]. SPECTROSCOPY AND SPECTRAL ANALYSIS, 2024, 44(07): 1877-1882. |
| [12] |
WANG Zi-xuan, YANG Miao, LIU Di-wen, MENG Bin, ZU En-dong*. The Study of Colored Freshwater Nucleated Pearl Via Raman Spectra and Chromaticity[J]. SPECTROSCOPY AND SPECTRAL ANALYSIS, 2024, 44(06): 1684-1688. |
| [13] |
LI Chang-ming1, GU Yi-fan2, ZHANG Hong-chen1, SONG Shao-zhong3*, GAO Xun2*. The Surface Enhanced Raman Spectroscopy Characteristics of Cyromazine Molecule Based on Density Function Theory[J]. SPECTROSCOPY AND SPECTRAL ANALYSIS, 2024, 44(06): 1566-1570. |
| [14] |
LIU Jing, YAO Yu-zeng*, FU Jian-fei, LI Zi-ning, HOU Ting-ting, ZHANG Yong-li. Micro-Raman Spectral Characteristics and Implication of Magnetite in Gongchangling Iron Mine[J]. SPECTROSCOPY AND SPECTRAL ANALYSIS, 2024, 44(06): 1697-1702. |
| [15] |
SI Min-zhen1, 2, WANG Min1, 2, LI Lun1, 2, YANG Yong-an1, 2, ZHONG Jia-ju3, YU Cheng-min3*. The Main Ingredients Analysis and Rapid Identification of Boletuses Based on Surface-Enhanced Raman Spectroscopy[J]. SPECTROSCOPY AND SPECTRAL ANALYSIS, 2024, 44(06): 1648-1654. |
|
|
|
|
