光谱学与光谱分析 |
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Optics Heterodyne Detection of the Autoionization State of Barium |
SUN Jiang1,SU Hong-xin1,WANG Yan-bang2,GUO Qing-lin1,ZUO Zhan-chun2,FU Pan-ming2 |
1. Physical Science & Technology College, Hebei University, Baoding 071002, China 2. Laboratory of Optical Physics, Insitute of Physics, Chinese Academy of Sciences, Beijing 100080, China |
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Abstract The autoionization state of barium was observed by optics heterodyne between three-photon resonant nondegenerated six-wave mixing (NSWM) and two-photon resonant nondegenerated four-wave mixing (NFWM). In this way,optics heterodyne spectrum of 6p3/219d autoionization state of barium was measured. The suppression and enhancement of the NFWM signal was observed which was caused by the quantum interference between NFWM and NSWM. Our method is a pure nonlinear optic technique. It has the advantages of excellent spatial signal resolution and simple optical alignment. Here two-photon resonant NFWM is used as local oscillation, while three-photon resonant NSWM signal is used as signal beam. Detection of autoionization states of Ba was achieved by changing the frequency of signal beam. The phase matching condition of this technique is not so stringent and can be achieved over a very wide frequency range, which is very difficult in the general six-wave mixing. Furthermore, the signal is coherent light. Optics heterodyne spectrum is a Doppler- free spectroscopy when the incident lasers have narrow bandwidths.
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Received: 2006-11-18
Accepted: 2007-03-06
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Corresponding Authors:
SUN Jiang
E-mail: hdsunjiang@163.com
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[1] WANG Yong-jing, ZHANG Han-hui, HUANG Chang-cang, et al(王永净, 张汉辉, 黄长沧, 等). Spectroscopy and Spectral Analysis(光谱学与光谱分析), 2006,26(2): 287. [2] ZHANG Dong-xian, ZHANG Hai-jun, LIN Xiao-feng, et al(张冬仙, 章海军, 林晓峰, 等). Spectroscopy and Spectral Analysis(光谱学与光谱分析), 2006, 26(3): 441. [3] JIN Chang-tai, WANG Xiu-lan(金昌泰,王秀兰). Spectroscopy and Spectral Analysis(光谱学与光谱分析), 1999,19(1): 5. [4] DU Hai, SHI Gui-zhen, HUANG Mao-cheng, et al(杜 海,史桂珍,黄茂成,等). Spectroscopy and Spectral Analysis(光谱学与光谱分析), 2000, 20(3): 260. [5] Cooke W E, Gallagher T F, Edelstein S A, et al. Phys. Rev. Lett., 1978, 40(3): 178. [6] Dai C D. Phys Rev. A, 1995, 52(6): 4416. [7] Eesley G L. Coherent Raman spectroscopy. Oxford: Pergamon Press, 1981. [8] Saha S K, Hellwarth R W. Phys. Rev. A, 1983, 27(2): 919. [9] JIA Suo-tang, DENG Shi-lan, QIN Li-juan, et al(贾锁堂,邓仕兰,秦莉娟,等). Spectroscopy and Spectral Analysis(光谱学与光谱分析), 1995,15(3): 27. [10] SUN Jiang, ZUO Zhan-chun, MI Xin, et al(孙 江,左战春,米 辛, 等). Chin. Phys. Sin.(物理学报), 2005, 54(1): 149. [11] SUN Jiang, ZUO Zhan-chun, GUO Qing-lin, et al(孙 江,左战春,郭庆林,等). Chin. Phys. Sin.(物理学报), 2006, 55(1): 221. [12] ZUO Zhan-chun, SUN Jiang, LIU Xia, et al. Phys. Rev. Lett.,2006, 97(11): 193904. [13] Turukhin A V, Sudarshanam V S, Shahriar M S. Phys. Rev. Lett., 2002, 88(1): 023602. |
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